As well as using the generator in contact or remote mode, I need to produce a periodic emf of a particular frequency and field strength. Is there any reason that I cant connect the output to a properly wound coil to create such a magnetic field?

Yes, this should work. Make sure you use magnet wire, which is copper wire insulated with enamel. Also, if the resistance of your coil is super low, you may need to add a resistor in series (say 50 ohm).

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